金属团簇反应性与软沉积
金属团簇层流反应与软沉积
工作组成员:程然、郜毅帆
气相团簇反应的研究通常有两个导向。一方面,旨在探索特定新物种的反应活性 (尤其是催化活性);另一方面,团簇科学的一个重要研究任务在于探寻不同于普通分子结构和价键相互作用的具有异常稳定性的团簇新物种。于此,团簇高气压充分多碰撞反应就显得尤其重要。本仪器可高效制备金属团簇,并发挥富压充分反应的优势,针对磁控溅射制备的各类金属团簇,实现其富压层流反应和定性定量质谱检测。
多离子层流反应管串联三重四极杆质谱系统 (MIFT-TQMS)
References
- Benben Huang; Hanyu Zhang; Wen Gan; Mengzhou Yang; Zhixun Luo*; Jiannian Yao, Nb12+——Niobespherene: a full-metal hollow cage cluster with superatomic stability and resistant to CO attack. Natl. Sci. Rev. 2022, DOI:10.1093/nsr/nwac197.
- Benben Huang, Haiming Wu, Mengzhou Yang, Zhixun Luo*, An integrated instrument of a tandem quadrupole mass spectrometer for cluster reaction and soft-landing deposition Rev. Sci. Instrum. 2022, in production.
- W. Gan; L. Geng; B. Huang; K. Hansen; Z. Luo, Dehydrogenation of diborane on small Nbn+ clusters. Phys. Chem. Chem. Phys. 2024, 26 (12), 9586-9592..
- Benben Huang; Wen Gan; Klavs Hansen; Zhixun Luo, What Determines the Drastic Reactivity of Nbn+ Clusters with Nitric Oxide under Thermalized Conditions? J. Phys. Chem. A 2022, 126 (29), 4801–4809.
- Z. Luo; Arthur C. Reber; Meiye Jia; William H. Blades; Shiv N. Khanna; A. W. Castleman, Jr., What determines if a ligand activates or passivates a superatom cluster? Chem. Sci. 2016, 7, 3067–3074.